English
聯系我們
網站地圖
郵箱
舊版回顧



蘇州納米所等在石墨烯氣凝膠領域取得進展

文章來源:蘇州納米技術與納米仿生研究所   發布時間:2019-05-10  【字號:     】  

  石墨烯氣凝膠,經由石墨烯片層三維搭接、組裝而來的石墨烯宏觀體材料,具有三維連續多孔網絡結構,表現出高比表面積、高孔隙率、優異導電性能及電化學行為,在能源存儲、傳感、吸附、復合材料等領域有重要應用前景。然而,目前常規石墨烯氣凝膠的三維組裝以石墨烯片層間的“面-面”局部搭接方式為主,進而形成具有三維無規連續多孔網絡。石墨烯片層間的這種“面-面”堆垛-搭接方式,是一種無規、隨機組裝,往往會使得部分石墨烯片層形成類石墨結構,造成石墨烯本征性能(如比表面積、力學、電學等)損失。此外,傳統石墨烯氣凝膠所具有的這種無規三維多孔網絡還引入高界面電阻及曲折離子通道問題,對電化學行為中的電荷-離子傳輸及有效電化學活性面積維持帶來負面影響,成為制約石墨烯材料在電化學能源器件中應用的瓶頸。因此,如何設計新的石墨烯組裝策略,制備高性能石墨烯氣凝膠材料,仍是一個重要挑戰。

  針對石墨烯氣凝膠目前存在的問題,中國科學院蘇州納米技術與納米仿生研究所研究員張學同領導的氣凝膠團隊通過“局部氧化刻蝕”在氧化石墨烯片層上進行造孔,獲得孔洞氧化石墨烯,隨后將孔洞氧化石墨烯與還原劑分散液高度濃縮,實現其液晶化,進一步經原位溶膠凝膠及超臨界干燥獲得各向異性“孔洞石墨烯”氣凝膠,如圖所示。所得各向異性“孔洞石墨烯”氣凝膠由孔洞石墨烯片層經有序排列而成,表現出規整的三維多孔網絡(規整的孔道/孔壁及孔壁上的大量微孔)、低密度(42-55 mg cm-3)、高導電性(~165 S m-1)、高比表面積(537~837 m2 g-1)等諸多優點。最后將該氣凝膠作為電極材料,輔以共晶混合物“水-甲酰胺”作為低溫電解液,構建出可在溫度低至零下40°C的環境中正常工作的柱狀低溫熱電化學池,表現出低離子傳輸阻力(15.7 Ω)及高輸出功率(3.6 W m-2)。當15個熱電化學池進行串聯組裝成器件時,可實現~2.1 V電壓的穩定輸出,在低溫能源器件應用中表現出重要應用前景。

  相關成果以High-Efficiency Cryo-Thermocells Assembled with Anisotropic Holey Graphene Aerogel Electrodes and a Eutectic Redox Electrolyte 為題發表在國際期刊《先進材料》(Advanced Materials20191901403)上。博士生李廣勇、碩士董大鵬及澳門大學教授洪果為論文共同第一作者,張學同與英國UCL教授宋文輝為論文共同通訊作者,合作者還包括中國科學技術大學教授閆立峰。論文工作獲得國家重點研發計劃、國家自然科學基金委、英國皇家學會-牛頓高級學者基金等資助。

  圖:各向異性“孔洞石墨烯”氣凝膠基本表征:氧化石墨烯片層的透射電鏡照片(a1)及氧化石墨烯液晶的偏光顯微鏡照片(b1),孔洞氧化石墨烯片層的透射電鏡照片(a2)及氧化石墨烯液晶的偏光顯微鏡照片(b2),氧化石墨烯及孔洞氧化石墨烯片層的拉曼光譜(c),各向異性“孔洞石墨烯”氣凝膠的光學照片(d)、掃描電鏡照片(ef)、力學(g)、電學(h)及比表面積數據(i)。




(責任編輯:葉瑞優)

附件:

專題推薦

相關新聞


© 1996 - 中國科學院 版權所有 京ICP備05002857號  京公網安備110402500047號  聯系我們

地址:北京市三里河路52號 郵編:100864

亿彩彩票www.yi543.com www.73km.com | www.033734.com | www.301439.com | pu14.com | 422835.com | www.fc97.com | www.23ih.com | www.0048.cc | www.88932.cc | www.077525.com | www.226922.com | www.365414.cc | www.587002.com | www.666721.com | www.790182.com | www.880160.com | 福利彩票www.99677g.com | www.8880.online | www.70626.com | www.356746.com | www.799181.com | 594150.com | 559595.com | 873702.com | www.cai5151.com | www.ng91.com | www.294.biz | www.114158.com | www.234915.com | www.357162.com | www.770998.com | www.798981.com | 392323.com | 288991.com | 356582.com | 奔驰彩票www.750966.com | www.kf59.com | www.2886.biz | www.9613.biz | www.62887.com | www.218690.com | www.315458.com | www.610540.com | www.769208.com | www.882716.com | www.99xz.com | www.47606.com | www.129509.com | www.831129.cc | www.933995.com | 146666.com | 982541.com | 827016.com | www.875026.com | www.vk6.com | www.s60.mobi | www.88bp.com | www.4989.org | www.97511.cc | www.777433.com | www.926781.com | www.974742.com | www.33hv.com | www.50323.com | www.099079.com | www.229635.com | www.291936.com | www.208391.com | www.356883.com | www.732583.com | www.872099.com | 华人彩票www.454589.com | www.87222.cc | www.179621.com | www.315682.com | www.374773.com | www.732306.com | 671620.com | 556594.com | 九五彩票www.95333w.com | www.mq97.com | www.26zo.com | www.0168.top | www.8292.biz | www.385658.com | www.661065.com | www.988813.com | 322845.com | 960465.com | 438143.com | 鑫亿彩www.196073.com | www.037116.com | www.ci42.com | www.52er.com | www.936.vip | www.55343.cc | www.497717.com | www.811447.com | www.877771.com | 292087.com | 503878.com | 623501.com | 手机购彩www.632599.com | www.qs51.cc | www.02ue.com | www.381.cn | www.26949.com | www.5be.com | 261776.com | www.ag59.cc | www.071589.com | www.136826.com | www.275342.com | www.379680.com | www.590631.com | www.651708.com | www.818142.com | www.870647.com | www.972840.com | 35351.com | 6626.com--6626.com | 69ja.com | 440679.com | 020455.com--020455.com | 金冠彩票www.49956p.com | www.fe13.com | www.m06.net | www.67fl.com | www.90pj.cc | www.5603.wang | www.22650.com | www.73367.cc | www.051125.com | www.076290.com | www.111786.com | www.353305.com | www.436323.com | www.794545.com | www.874752.com | 500117.com | 025362.com | 362.net | 214389.com | 68彩票www.68689p.com | 誉信彩票www.757q.com | 大赢家彩票平台www.810521.com | www.hv83.com | www.94db.com | www.81422.cc | www.165876.com | www.559341.com | www.633637.com | www.734608.com | www.824877.com | www.889493.com | www.925633.com | www.937663.com | 33552.com | www.069335.com | www.126759.com | www.169611.com | www.338263.com | www.433370.com | www.521133.com | 690097.com | 909513.com | 212005.com | 博友彩www.371p.cc | www.hh21.com | www.xc67.com | www.nx60.com | www.44ub.com | www.022278.com | www.122807.com | www.308081.com | www.333012.com | www.354119.com | www.731451.com | www.813086.com | www.967940.com | 632030.com | 299508.com | www.58531111.com | sb36.com | lehu666.vip | 939380.com | 8816彩票www.8816x.com | 大赢家彩票网www.83033p.com | www.cp0305.com | www.sp32.com | www.096.bid | www.989275.com | www.999079.com | www.748244.com | 397106.com | po74.com | 90158.cc | 322510.com | 033643.com | 610329.com | www.cp0570.com | www.63sb.com | www.798596.com | 93397.com | 878065.com | 881436.com | 970622.com | 254827.com | 304499.com | www.cai52.cc | www.dk25.com | www.27hs.com | www.34gu.com | www.47uv.com | www.93vl.com | www.876.org | www.6266.in | www.00791.cc | www.22135.com | www.018060.com | www.109422.com | www.380676.com | www.691270.com | www.733619.com | www.814844.com | www.822480.com | www.837883.com | www.858981.com | 144464.com | 531792.com | www.57ii.com | www.99oe.com | www.7469.vip | www.182521.com | www.926116.com | www.949546.com | www.961615.com | www.970218.com | 587095.com | E彩堂www.9818j.cc | www.78pz.cc | www.9614.com | www.03876.com | www.27183.com | www.215593.com | www.207115.com | www.250159.com | www.400233.com | 662424.com | 038101.com | 598508.com | www.60598.com | www.080101.com | www.098889.com | www.371771.com | www.571762.com | www.989979.com | www.984527.com | www.950201.com | www.957837.com | www.947336.com | www.932127.com | 915250.com | 486179.com | 721602.com | 381421.com | 819411.com | 必发彩票www.8970.com | 天吉彩票www.9205g.com | 好彩www.60123r.com | 双彩网www.506906.com | 13e彩票www.816142.com | www.cp4345.com | www.26359.cc | www.37172.cc | www.12318.com | www.11902.com | www.40894.com | www.41936.com | www.13211.cc | www.15717.com | www.19255.cc | www.15915.cc | www.8438.com | www.8833.top | www.7532.com | www.23922.com | www.75320.com | www.032763.com | www.058345.com | www.079068.com | www.085080.com | www.073034.com | www.107053.com | www.118040.com | www.096067.com | www.139621.com | www.457335.com | www.505270.com | www.521406.com | www.500940.com | www.461706.com | www.435613.com | 595315.com | 717170.com | 84xi.com | 大赢家彩票网www.54400j.com | 凤凰彩票www.77802d.com | 500彩票www.202434.com | 购彩堂www.113438.com | 500彩票www.26299w.com | 九五彩票www.95999w.com | 68彩票www.68689c.com | 六福彩票www.66ffk.com | 496883.com | 241234.cc | 彩票坊www.022tw.cc | 99彩票www.99048.cc | 博亿彩票www.656by.com | 625287.com | www.3160.vip | www.3657.com | www.932.hk | www.1090.cn | www.9740.loan | www.30271.com | www.36985.com | www.21718.com | www.47399.com | www.019737.com | www.070594.com | www.082071.com | www.070991.com | www.048809.com | www.040481.com | www.042352.com | www.43674.com | www.37827.com | www.22956.cc | www.115128.com | www.474591.com | www.499304.com | www.429877.com | www.357069.com | www.539794.com | www.520247.com | www.669936.com | www.625848.com | www.635256.com | www.867330.com | www.991628.com | www.949816.com | 484565.com | 432026.com | j15.me | 218909.com | 974870.com | 356432.com | 309652.com | 7093.com | www.088878.cc | www.089139.com | www.091666.com | www.065289.com | www.50096.cc | www.050082.com | www.037083.com | www.254009.com | www.295931.com | www.261445.com | www.275655.com | www.716785.com | www.685863.com | www.711735.com | www.682186.com | www.628930.com | www.876626.cc | 011694.com | 149291.com | 665012.com | www.lf27.com | www.j83.com | www.ag1.com | www.74qp.com | www.75vu.com | www.34au.com | www.sb76.com | www.bi32.com | www.3826.vip | www.0360.cc | www.8580.org | www.5451.top | www.0304.loan | www.6628.net | www.5729.bid | www.6409.cm | www.0591.org | www.5077.xyz | www.1855.tv | www.4593.vip | www.5934.cc | www.9745.com | www.63217.com | www.123481.cc | www.093940.com | www.065912.com | www.022357.com | www.120204.com | www.061173.com | www.043247.com | www.001069.com | www.69521.com | www.039934.com | www.78187.com | www.017234.com | www.72418.com | www.084900.com | www.036883.com | www.78033.cc | www.217326.com | www.178908.com | www.580070.com | www.517650.com | www.362631.com | www.708618.com | www.777793.com | 236444.com | 345864.com | www.954739.com | 654463.com | 258327.com | 679249.com | www.507571.com | www.349816.com | www.171279.com | www.558955.com | www.394967.com | www.772484.com | www.612624.com | www.550450.com | www.354644.com | www.220043.com | www.339452.com | www.268036.com | www.172588.com | www.337294.com | www.166277.com | www.065308.com | www.73368.cc | www.66236.cc | www.52471.com | www.36354.com | www.6033.org | www.v24.in | 964963.com | www.936388.com | www.572162.com | www.455026.com | www.443388.com | www.292428.com | www.154321.cc | www.095362.com | www.35292.cc | www.94gv.com | www.dk62.com | 吉利彩票www.80075h.com | 678906.cc | 982470.com | 871928.com | www.886536.com | 151039.com | www.917730.com | www.705272.com | www.830916.com | www.929646.com | www.726338.com | www.691665.com | www.829217.cc | www.744482.com | www.574182.com | www.375315.com | www.235221.com | www.085320.com | www.98667.cc | www.9440.vip | www.11351.com | www.82xm.com | www.37mk.com | www.pu0.com | 165104.com | 986427.com | www.963485.com | www.799744.com | www.618129.com | www.553599.com | www.331212.com | www.177507.com | www.087759.com | www.46505.com | www.3883.vip | www.00yu.com | 七星乐www.535666a.com | 468489.com | 814011.com | 367601.com | 033365.com | www.821787.com | www.698787.com | www.528882.com | www.331019.com | www.116862.com | www.062897.com | www.32638.com | www.7666.live | www.18vn.com | 购彩票www.c5907.com | 650234.com | 亿龍彩票www.1368n.cc | 616493.com | www.970499.com | www.850663.com | www.757793.com | www.909271.com | www.777367.com | www.762523.com | www.534715.com | www.313330.com | www.249887.com | www.051672.com | www.25572.cc | www.99pe.com | www.wz93.cc | www.723123.com | 141959.com | www.nw96.com | 大赢家彩票网www.178532.com | 066092.com | www.967426.com | www.887438.com | www.862586.com | www.948308.com | www.889819.com | www.741615.com | www.704822.com | www.590008.com | www.650791.com | www.581229.com | www.479321.com | www.346818.com | www.249678.com | 492298.com | 912085.com | www.949212.com | www.926153.com | www.763058.com | www.959335.com | www.880360.com | www.984289.com | www.884599.com | www.865734.com | www.905803.com | www.758627.com | www.607899.com | www.484448.com | www.295941.com | www.225778.com | www.413101.com | www.631965.com | www.996848.com | www.872983.com | www.798812.com | www.981714.com | www.863788.com | www.945799.com | www.659746.com | www.791823.com | www.336977.com | www.35472.com | www.3725.pw | www.221660.com | www.895277.com | www.739658.com | www.585103.com | www.412316.com | www.435463.com | www.380528.com | www.297990.com | www.732678.com | www.520179.com | www.660647.com | www.605708.com | www.571184.com | www.572763.com | www.628663.com | www.651104.com | www.620638.com | www.637297.com | www.799962.com | www.589813.com | www.551733.com | www.494808.com | www.356940.com | www.305832.com | www.313232.com | www.155736.com | www.115986.com | www.83650.com | www.2018ptw.com | 701518.com | www.952065.com | www.773725.com | www.719327.com | www.784735.com | www.622570.com | www.650741.com | www.641558.com | www.672324.com | www.505536.com | www.370831.com | www.336068.com | www.291028.com | www.161399.com | www.177430.com | www.309048.com | www.169704.com | www.135352.com | www.102227.com | www.66015.cc | www.66003.cc | www.38297.cc | www.2556.in | www.2088.love | www.0475.loan | www.95rf.com | www.79qq.com | www.le89.com | www.022454.com | www.31189.com | www.1048.xyz | www.345.cm | www.t90.cn | www.jr88.com | www.nn6.com | 652339.com | 894929.com | www.323362.com | 310306.com | 768337.com | 168590.com | www.966473.com | www.872955.com | www.874901.com | www.770453.com | www.624001.com | www.944365.com | www.731942.com | www.576490.com | www.443446.com | www.232719.com | www.105146.com | www.88539.cc | www.6480.net | www.74ad.com | www.25rp.com | www.fw23.com | 华人彩票www.hr1888.com | 433537.com | 268009.com | 55510.com | www.891120.com | www.815969.com | www.678787.com | www.613062.com | www.716155.com | www.599306.com | www.386676.com | www.299807.com | www.595432.com | www.449995.com | www.494808.com | www.460692.com | www.247312.com | www.110493.com | www.77816.com | www.081047.com | www.33210.cc | www.0440.cc | www.84ko.com | www.yy10.com | www.om51.com | 众乐彩票www.389344.com | 674929.com | 167456.com | www.971296.com | www.786196.com | www.664246.com | www.640515.com | www.345848.com | www.202377.com | www.508940.com | www.324624.com | www.140135.com | www.069601.com | www.43577.com | www.2044.cm | www.537.net | www.4066.xyz | www.09uy.com | 500万彩票www.96386k.com | 42tx.com | 604139.com | 144478.com | www.950849.com | 065650.com | www.922652.com | www.759213.com | www.535791.com | www.635785.com | www.748596.com | www.989651.com | www.891811.com | www.691543.com | www.511271.com | www.298693.com | www.129719.com | www.206603.com | www.085216.com | www.121077.com | www.022945.com | www.25319.cc | www.2151.space | www.9968.site | www.xb96.com | 凤凰彩票www.77801i.com | 743178.com | cp450.cc | 303643.com | 6373.biz | www.943738.com | www.909703.com | www.709555.com | www.971367.com | www.781336.com | www.776205.com | www.564912.com | www.438377.com | www.280405.com | www.075070.com | www.124656.com | www.77167.cc | www.094507.com | www.135000.cc | www.103805.com | www.198634.com | www.092144.com | www.58920.com | www.049035.com | www.55048.cc | www.58656.com | www.3310.tv | www.68358.cc | www.24433.cc | www.87hk.com | www.nj90.com | www.ca4.cc | 511274.com | 201255.com | www.995836.com | www.843422.com | www.972541.com | www.752671.com | www.577441.cc | www.375195.com | www.258849.com | www.034961.com | www.6909.vip | www.zf04.com | 992768.com | 931787.com | www.946857.com | www.682575.com | www.518877.com | www.301789.com | www.156550.com | www.229655.com | www.088439.com | www.147169.com | www.73381.cc | www.3893.com | www.ny32.com | 126彩票网www.126ll.com | 326020.com | www.913150.com | www.610506.com | www.458371.com | www.170739.com | www.092234.com | www.06378.com | www.901.vip | www.2507.org | www.lg96.com | 风之彩www.99fzc.com | 081084.com | www.916014.com | www.823204.com | www.569458.com | www.302751.com | www.033054.com | www.100720.com | www.217635.com | www.053516.com | www.6540.in | www.cp0408.com | 819066.com | www.957212.com | www.668577.com | www.379653.com | www.321302.com | www.192730.com | www.156879.com | www.35705.com | www.24ht.com | 458640.com | 777966.com | www.827742.com | www.533761.com | www.203722.com | www.71227.com | www.1411.xyz | www.36ea.com | 冠赢彩票www.610330.com | www.jd31.com | 64578.com | 845549.com | www.872863.com | www.832036.com | www.688904.com | www.528234.com | www.221775.com | www.190127.com | www.051835.com | www.6612.cc | www.ls04.com | 711308.com | 123593.com | www.765456.com | www.506319.com | www.185376.com | www.039566.com | www.4984.vip | www.12cf.com | 彩客网www.801876.com | 684353.com | www.876360.com | www.905687.com | www.560022.com | www.251382.com | www.80378.com | www.65si.com | 964075.com | www.880219.com | www.966871.com | www.666170.com | www.379273.com | www.067655.com | www.6930.top | www.lr86.com | 390197.com | www.996913.com | www.696799.com | www.366675.com | www.593812.com | www.433619.com | www.232456.com | www.038610.com | www.3606.vip | www.cp3988.com | 954912.com | www.856358.com | www.718921.com | www.413315.com | www.352700.com | www.365357.cc | www.220660.com | www.72738.com | www.03931.com | www.c23.vip | 378322.com | 732696.com | www.888827.com | www.660356.com | www.520851.com | www.392333.com | www.570268.com | www.233042.com | www.59911.com | www.792.cc | www.sh69.com | www.nv28.com | 329692.com | www.977466.com | www.633826.com | www.637393.com | www.341844.com | www.061044.com | www.3125.com | www.rl61.com | 580618.com | 00040.cc | www.664599.com | www.614626.com | 229096.com | www.882586.com | www.830398.com | www.518104.com | www.178263.com | www.92015.com | www.5525.wang | www.91tw.com | 997049.com | 7359.biz | www.736587.com | www.396694.com | www.280022.com | www.009079.com | www.95ug.com | www.872096.com | www.968514.com | www.451511.com | www.381649.com | www.381540.com | www.183857.com | www.72414.com | www.83sb.com | 73684.com | www.999895.com | www.623777.com | www.477216.com | www.414437.com | www.071815.com | www.7312.bid | www.wq9.cc | 359079.com | www.894532.com | www.621248.com | www.621493.com | www.655612.com | www.737378.com | www.553260.com | www.175111.cc | www.64403.com | www.57597.cc | www.61qd.com | www.wb10.com | 彩乐乐www.cll168.com | k88888.com | www.779851.com | www.392796.com | www.211172.com | www.24461.com | www.xm57.com | 819748.com | www.876422.com | www.747483.com | www.550169.com | www.218596.com | www.48968.com | www.0332.cm | www.py90.com | cai1100.com | www.886326.com | www.736725.com | www.422787.com | www.365706.cc | www.081706.com | www.1215.cc | www.if83.com | 463678.com | www.840337.com | www.786555.com | www.376875.com | www.433049.com | www.057308.com | www.0431.love | www.fi63.com | 034747.com | www.857027.com | www.546855.com | www.180108.com | www.015428.com | www.4233.top | www.cp3211.com | 022816.com | www.774575.com | www.348337.com | www.110418.com | www.06321.cc | www.ik94.com | 568476.com | www.925505.com | www.581684.com | www.235282.com | www.11563.com | www.iu87.com | 914.net | www.889739.com | www.503731.com | www.107313.com | www.6119.top | www.0qu.com | 940062.com | www.cp884.com | bk73.com | www.730997.com | www.365340.com | www.051323.com | www.351.pw | www.cai5055.com | 979092.com | 879031.com | www.708209.com | www.325587.com | www.137302.com | www.35533.com | www.038.org | 金掌柜www.83993w.com | www.966973.com | www.571595.com | www.544718.com | www.138897.com | www.12412.cc | www.ip24.com | www.cj10.com | 806918.com | www.788261.com | www.399836.com | www.096323.com | www.056155.com | www.09628.com | www.im25.com | 33408.cc | www.762719.com | www.328602.com | www.86477.cc | www.626.red | www.36rq.com | www.kn84.com | 549563.com | www.872328.com | www.572299.com | www.185229.com | www.9874.cn | www.au40.com | 039803.com | www.990659.com | www.659354.com | www.721675.com | www.411295.com | www.173295.com | www.113241.com | www.9521.loan | www.zs46.com | www.cr11.cc | 070929.com | www.995842.com | www.693276.com | www.383076.com | www.253846.com | www.284226.com | www.86299.com | www.83tw.com | 乐盈彩票www.88kcw.com | 374212.com | www.782552.com | www.659483.com | www.679213.com | www.377159.com | www.380806.com | www.106993.com | www.7331.net | www.if85.com | 506212.com | www.930294.com | www.590008.com | www.262157.com | www.058610.com | www.008325.com | www.0746.love | www.o47.net | 620095.com | www.953211.com | www.613117.com | www.449342.com | www.137014.com | www.63607.com | www.5188.space | www.u33.club | 990832.com | 557556.com | www.728282.com | www.849383.com | www.718188.com | www.405711.com | www.208013.com | www.98101.com | www.28464.com | www.zg35.com | ih61.com | 551550.com | 085841.com | www.826253.com | www.559649.com | www.285220.com | www.480824.com | www.123418.cc | www.5013.vip | www.tk82.com | 817224.com | www.879126.com | www.698085.com | www.394780.com | www.058760.com | www.334655.com | www.266591.com | www.79111.com | www.33903.com | www.35of.com | 858324.com | 98775.com | www.818584.com | www.639301.com | www.765475.com | www.525066.com | www.209333.com | www.185785.com | www.77215.cc | www.06969.com | www.rb72.com | 850113.com | www.912032.com | www.571956.com | www.300019.com | www.0516.live | www.w88.me | 175317.com | www.977083.com | www.670102.com | www.289366.com | www.161346.com | www.222723.com | www.5354.biz | www.fc52.com | 369468.com | www.775259.com | www.431432.com | www.056543.cc | www.01po.com | 748889.com | www.779060.com | www.381538.com | www.112081.com | www.9662.cc | 豪彩VIPwww.960883.com | www.ea84.com | www.499262.com | www.967034.com | www.803789.cc | www.561151.com | www.445228.com | www.120486.com | www.123483.com | www.717.space | www.uc01.cc | 984395.com | www.736537.com | www.324782.com | www.080177.com | www.1900.website | www.9398.biz | www.bh0.com | 563053.com--563053.com | www.696232.com | www.580269.com | www.158117.com | www.099556.com | www.1064.xyz | 吉彩www.602582.com | www.979604.com | www.560938.com | www.128646.com | www.9995.hk | www.fd16.com | 4258.biz | www.675608.com | www.168385.com | www.9976.top | www.bh08.com | www.994160.com | www.963416.com | www.630097.com | www.259905.com | www.8225.in | www.cai217.com | www.958640.com | www.583139.com | www.216037.com | www.7197.biz | GO彩www.chi59.com | www.954283.com | www.506123.com | www.019353.com | www.0058.vip | www.3875.top | 348890.com | www.926337.com | www.464993.com | www.048282.com | www.4530.com | 612389.cc | www.941829.com | www.501675.com | www.017270.com | www.u68.com | 347641.com | www.775765.com | www.333144.com | www.275132.com | www.23394.com | 500彩票www.50052f.com | www.958401.com | www.491177.com | www.86400.cc | www.65py.com | 369794.com | www.835611.com | www.881327.com | www.521202.com | www.170875.com | www.000276.com | www.6454.com | www.cp5659.com | 979028.com | www.995683.com | www.607210.com | www.349422.com | www.42072.com | www.xg26.com | 539671.com | www.962528.com | www.539010.com | www.125372.com | www.45576.com | www.ry38.com | 562357.com | www.954256.com | www.562559.com | www.188005.com | www.11879.com | www.62bl.com | 931252.com | 397333.com | www.671979.com | www.242266.com | www.25578.cc | www.40uk.com | 579539.com | www.984601.com | www.572629.com | www.137608.com | www.33170.com | www.63na.com | 24453.com | www.920982.com | www.490433.com | www.041682.com | www.64fe.com | 308499.com | 579210.com | www.751676.com | www.326553.com | www.38820.cc | www.06yv.com | 655552.com | www.868912.com | www.668825.cc | www.262360.com | www.125567.com | www.072701.com | www.2532.org | 凤凰彩票www.66652f.com | www.972542.com | www.708271.com | www.294744.com | www.039797.com | www.54sy.com | 716792.com | www.900016.cc | www.553053.com | www.785653.com | www.491166.com | www.078765.com |